Date: Tue, 12 Sep 2006 22:25:53 +0530 (IST)

From: E. Arunan <arunan@ipc.iisc.ernet.in>

To: Task Group

Subject: H bond

 

Dear Colleagues,

I have updated the webpage with all the recent emails

and also some comments from experts outside the task

group. For your information the following webpage has

all the details.

http://ipc.iisc.ernet.in/~arunan/iupac/

This email is slightly longish.

I would like to know if we have a consensus on some

of the following statements. Kindly send your views

sometime this week:

 

1) There is no unique physical force that can be

   described as 'hydrogen bonding'

2) Electron deficient hydrogen: I should have pointed

   out Dannenberg's objection to these words in my

   earlier email. Would 'electropositive' or 'a hydrogen

   atom that carries a partial postive charge' be

   acceptable to all members, especially Scheiner and

   Dannenberg. Do all hydrogen bonds involve some X-H

   groups that has a dipole moment with H being the

   positive end?

3) Rosenberg points out that enhancement of IR intensity

   is a defining characterestic of H bond. There are

   some blue-shifting H bonds that show reduction

   in X-H intensity.

4) In the F-(H2) (fluoride ion complexed with H2), the

   structure is linear. Though H2 has no dipole or electro-

   positive Hydrogen atom, I think in the F(-)H-H complex

   the H bonded to F will acquire a partial positive

   charge. Would this qualify as a H bonded complex?

5) Should we propose London molecules as a new terminology

   for molecules that are primarily bound by dispersive

   forces? There could be 'H bonded complexes' that may

   come under this list and I don't see that as a problem.

6) Can van der Waals forces be used to describe all

   intermolecular (non bonded intra-molecular) interactions?

   Scheiner and I had some interesting exchange on this

   issue.

 

I welcome your comments.

with best regards,

Arunan.